Engineered Defects in Wide Band-gap Semiconductors for Single-spin Sensing and Computation

By Abram Falk

Institute for Molecular Engineering, University of Chicago, Chicago, IL

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Abstract

While generally considered undesirable in traditional electronic devices, semiconductor defects can confine isolated electronic spins and act as nanoscale, single-spin memory registers. Alongside research efforts focusing on nitrogen-vacancy centers in diamond, an alternative approach seeks to identify and control new spin systems in new materials, a strategy that could ultimately lead to “designer” spins with tailored properties for future quantum photonics and nanoscale sensing applications. Using infrared light at near-telecom wavelengths, I will show that spin states in silicon carbide exhibit long quantum coherence times that persist up to room temperature. I will also discuss new strategies for generating coherent spin interactions at the nanoscale using defects in inequivalent lattice sites (Fig. 1), as well as resonant electric and strain fields. Together with the availability of industrial scale crystal growth and advanced microfabrication, wide-gap semiconductors are promising platforms for room-temperature quantum technologies that merge spin degrees of freedom with electronics and photonics.

Interacting spin states based on inequivalent defects in SiC
Fig. 1. Interacting spin states based on inequivalent defects in SiC

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  • Abram Falk (2014), "Engineered Defects in Wide Band-gap Semiconductors for Single-spin Sensing and Computation," https://nanohub.org/resources/20739.

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Birck Technology Center, Room 1001, Purdue University, West Lafayette, IN

Engineered Defects in Wide Band-gap Semiconductors for Single-spin Sensing and Computation
  • Engineered defects in wide band-gap semiconductors for single-spin sensing and computation 1. Engineered defects in wide ban… 0
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  • Crystal Vaccum 2. Crystal Vaccum 132.0653987320654
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  • Single-pin optical adressability 3. Single-pin optical adressabili… 152.5191858525192
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  • Engineered defects in wide gap semiconductors 4. Engineered defects in wide gap… 234.5679012345679
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  • Wide band-gap semiconductors in industry 5. Wide band-gap semiconductors i… 273.87387387387389
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  • Deep-level defects: artificial atoms 6. Deep-level defects: artificial… 372.93960627293961
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  • Importance of spin coherence for quantum information and nanoscale sensing 7. Importance of spin coherence f… 518.75208541875213
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  • Spin qubits and power electronics 8. Spin qubits and power electron… 663.86386386386391
    00:00/00:00
  • Engineered defects in wide gap semiconductors 9. Engineered defects in wide gap… 750.05005005005012
    00:00/00:00
  • Diamond NV centers: optically addressable single spins 10. Diamond NV centers: optically … 757.25725725725727
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  • Experimentally observing NV centers in diamond 11. Experimentally observing NV ce… 942.70937604270944
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  • Room-temperature optical excitation and phonon relaxation: a quantum process? 12. Room-temperature optical excit… 1038.8388388388389
    00:00/00:00
  • Room-temperature optical excitation and phonon relaxation: a quantum process? 13. Room-temperature optical excit… 1231.2312312312313
    00:00/00:00
  • Towards diamond NV-center technology 14. Towards diamond NV-center tech… 1403.7037037037037
    00:00/00:00
  • Diamond challenges: from proofs of principle to practical technology? 15. Diamond challenges: from proof… 1656.1895228561896
    00:00/00:00
  • Engineered defects in wide gap semiconductors 16. Engineered defects in wide gap… 1755.5889222555891
    00:00/00:00
  • SiC: leveraging advanced semiconductor capabilities towards single-spin technologies 17. SiC: leveraging advanced semic… 1757.1571571571571
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  • SiC and diamond: complementary hosts for spin qubits 18. SiC and diamond: complementary… 1822.0553887220556
    00:00/00:00
  • Crystal polymorphism in SiC 19. Crystal polymorphism in SiC 2081.0477143810476
    00:00/00:00
  • Engineering defects in SiC 20. Engineering defects in SiC 2210.8441775108445
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  • Engineering patterned spin arrays in SiC 21. Engineering patterned spin arr… 2286.4864864864867
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  • Neutral divacancies and related states in SiC 22. Neutral divacancies and relate… 2359.1257924591259
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  • Optically detected magnetic resonance 23. Optically detected magnetic re… 2513.1131131131133
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  • Optically detected magnetic resonance in SiC 24. Optically detected magnetic re… 2595.6956956956956
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  • Long-lived spin coherence 25. Long-lived spin coherence 2684.9182515849184
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  • Engineered defects in wide gap semiconductors 26. Engineered defects in wide gap… 2849.2158825492161
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  • Electrically and mechanically tunable electron spins in SiC 27. Electrically and mechanically … 2864.9983316649987
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  • Mechanically tunable electron spins in SiC 28. Mechanically tunable electron … 2933.2332332332335
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  • Understanding defect properties with ab-initio calculations 29. Understanding defect propertie… 2975.3086419753085
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  • AC electric fields: electrically driven spin resonance 30. AC electric fields: electrical… 3108.341675008342
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  • AC electric fields: electrically driven spin resonance 31. AC electric fields: electrical… 3144.3109776443112
    00:00/00:00
  • Coherent magnetic dipole interactions between inequivalent spins 32. Coherent magnetic dipole inter… 3191.0243576910243
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  • Engineered defects in wide gap semiconductors 33. Engineered defects in wide gap… 3275.608942275609
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  • Outlook: Coupling spins coupled to photonic crystals and mechanical resonators 34. Outlook: Coupling spins couple… 3281.4147480814149
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  • Outlook: Microscope-free platforms for single-spin devices 35. Outlook: Microscope-free platf… 3425.5922589255924
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  • Outlook: Spin-nanostructure interfaces 36. Outlook: Spin-nanostructure in… 3480.5472138805471
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  • Outlook: New optically addressable spins 37. Outlook: New optically address… 3523.6236236236236
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  • Acknowledgments 38. Acknowledgments 3606.2062062062064
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  • Conclusions 39. Conclusions 3616.3830497163831
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