Nanoscale NMR Studies of Topological Insulators, Crystalline Insulators and Dirac Semimetals

By Louis Bouchard

Department of Chemistry and Biochemistry, University of California Los Angeles, Los Angeles, CA

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Abstract

In recent years the emergence of gapless topologically protected edge states in the solid state has led to searches for new phases of condensed matter in new and existing materials. For example, some thermoelectrics and Kondo insulators have been shown to be topological insulators. The protected edge states in topological insulators are due to the combination of spin-orbit coupling and time-reversal invariance. Examples of exotic phenomena include the quantum anomalous Hall effect, fractional quantum anomalous Hall effect, topological superconductor, fractional time-reversal invariance, topological Kondo insulator, topological crystalline insulator and the topological magneto-electric effect. However, interesting properties of topological materials are found at edges and interfaces, making them challenging to study from the experimental standpoint. In this talk, we will review recent advances in experimental techniques to study the electronic and magnetic properties of such topological materials. Among the novel techniques, we shall discuss radioactive ion beam spectroscopy and nuclear magnetic resonance. Our group has been carrying out experiments at TRIUMF using low energy spin-polarized lithium-8 ion beams to resolve properties as function of depth, with nanoscale resolution. Such studies reveal substantial modulations of the metallic character of these materials at those length scales. Studies of material defects in the bulk will also be discussed. Ultimately, the development of new experimental methods is expected to lead to not only insight for improving material properties but may also enable the development of composite materials with optimized properties.

Bio

Louis Bouchard Dr. Bouchard obtained a bachelor's degree in physics and business management from McGill University in Montréal, Canada, a Master's degree in medical biophysics from the University of Toronto and a Ph.D. in Chemistry from Princeton University. His doctoral dissertation explores the use of multiple quantum coherence and long-range dipolar interactions in condensed matter to characterize heterogeneous material microstructure. During his stay in the laboratory of Alex Pines at the University of California, Berkeley he developed novel approaches and methodologies to portable, low-field NMR and MRI, microfluidics and hyperpolarization methods to the study of chemical reactions. He joined the UCLA faculty during the summer of 2008 to pursue research in physical chemistry.

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Cite this work

Researchers should cite this work as follows:

  • Louis Bouchard (2019), "Nanoscale NMR Studies of Topological Insulators, Crystalline Insulators and Dirac Semimetals," https://nanohub.org/resources/30532.

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Time

Location

Physics, Room 203, Purdue University, West Lafayette, IN

Tags

Nanoscale NMR Studies of Topological Insulators, Crystalline Insulators and Dirac Semimetals
  • Nanoscale NMR studies of topological insulators, 1. Nanoscale NMR studies of topol… 0
    00:00/00:00
  • TODAY's TOPICS 2. TODAY's TOPICS 61.89522856189523
    00:00/00:00
  • Electrons In Crystals 3. Electrons In Crystals 95.662328995662335
    00:00/00:00
  • Electrons In Crystals 4. Electrons In Crystals 112.77944611277945
    00:00/00:00
  • Band Theory of Solids 5. Band Theory of Solids 116.28294961628295
    00:00/00:00
  • Macroscopic Solid: Add e- Fills Bands 6. Macroscopic Solid: Add e- Fill… 132.03203203203205
    00:00/00:00
  • 2D Metal in Magnetic Field 7. 2D Metal in Magnetic Field 141.70837504170839
    00:00/00:00
  • Topology: 1D Edge States Conduct Current 8. Topology: 1D Edge States Condu… 174.70804137470805
    00:00/00:00
  • TI & Topological Invariant 9. TI & Topological Invariant 179.11244577911245
    00:00/00:00
  • TKNN: Topological Invariant for QHE 10. TKNN: Topological Invariant fo… 213.04637971304638
    00:00/00:00
  • Are Landau levels the only system with TKNN ν≠0? 11. Are Landau levels the only sys… 219.45278611945278
    00:00/00:00
  • 2D TI: Quantum Spin Hall Effect - Experiments 12. 2D TI: Quantum Spin Hall Effec… 224.12412412412414
    00:00/00:00
  • 3D TIs: From Theory to Experiments 13. 3D TIs: From Theory to Experim… 239.83983983983984
    00:00/00:00
  • Experimental domonstrations 14. Experimental domonstrations 268.70203536870207
    00:00/00:00
  • Requirements for Ideal TI 15. Requirements for Ideal TI 369.76976976976977
    00:00/00:00
  • Goal: Probe n- and p-Type Materials, With Defects, up to RT 16. Goal: Probe n- and p-Type Mate… 392.39239239239242
    00:00/00:00
  • TODAY's TOPICS 17. TODAY's TOPICS 508.67534200867539
    00:00/00:00
  • TI Bulk Properties 18. TI Bulk Properties 514.78144811478148
    00:00/00:00
  • E-N Hyperfine Interaction 19. E-N Hyperfine Interaction 603.57023690357028
    00:00/00:00
  • Orbital Hyperfine Interaction (TI) 20. Orbital Hyperfine Interaction … 1068.4684684684685
    00:00/00:00
  • KORRINGA LAW IN Bi2Te3 21. KORRINGA LAW IN Bi2Te3 1285.6189522856189
    00:00/00:00
  • NEGATIVE KNIGHT SHIFT 22. NEGATIVE KNIGHT SHIFT 1784.8515181848516
    00:00/00:00
  • Nuclear Quadrupolar Central Transition 23. Nuclear Quadrupolar Central Tr… 2061.8952285618952
    00:00/00:00
  • Isotopic Ratio & Korringa Law 24. Isotopic Ratio & Korringa Law 2167.867867867868
    00:00/00:00
  • βNMR STUDIES 25. βNMR STUDIES 2424.090757424091
    00:00/00:00
  • M1352: TI/OI Thin-Film Heterostructure 26. M1352: TI/OI Thin-Film Heteros… 2638.7721054387721
    00:00/00:00
  • Knight Shift Measures Carrier Density 27. Knight Shift Measures Carrier … 2727.1271271271271
    00:00/00:00
  • M1352: Knight Shift, Hyperfine Constant, Local Carrier Concentration 28. M1352: Knight Shift, Hyperfine… 2858.5251918585254
    00:00/00:00
  • Depth-Resolved Magnetic Properties 29. Depth-Resolved Magnetic Proper… 2973.3733733733734
    00:00/00:00
  • Nanoscale Findings From Depth Profiling 30. Nanoscale Findings From Depth … 3094.4277610944278
    00:00/00:00
  • topological crystalline insulatorS 31. topological crystalline insula… 3368.868868868869
    00:00/00:00
  • ARPES of Pb1-xSnxSe, x=10-40% 32. ARPES of Pb1-xSnxSe, x=10-40% 3396.62996329663
    00:00/00:00
  • CD vs T, Pb1-xSnxSe, x=20% 33. CD vs T, Pb1-xSnxSe, x=20% 3413.6803470136806
    00:00/00:00
  • Spin Dynamics and BI 34. Spin Dynamics and BI 3423.18985652319
    00:00/00:00
  • Surface State like Conductive Metal 35. Surface State like Conductive … 3469.4694694694695
    00:00/00:00
  • Field-Depending Korringa Process 36. Field-Depending Korringa Proce… 3489.78978978979
    00:00/00:00
  • Knight Shift @ Surface Reveal Gapless Semiconductor 37. Knight Shift @ Surface Reveal … 3495.8625291958629
    00:00/00:00
  • Topological Dirac Semimetals 38. Topological Dirac Semimetals 3525.7590924257593
    00:00/00:00
  • Evolution of non-trivial Fermi Surface Features 39. Evolution of non-trivial Fermi… 3531.731731731732
    00:00/00:00
  • Magnetic spin-olattice relaxaction 40. Magnetic spin-olattice relaxac… 3577.711044377711
    00:00/00:00
  • SUMMARY 41. SUMMARY 3612.345679012346
    00:00/00:00
  • Contributors: 42. Contributors: 3684.7514180847515
    00:00/00:00
  • acknowledgments 43. acknowledgments 3688.6886886886887
    00:00/00:00